First proof-of-principle experiment with the post-accelerated isotope separator on-line beam at BRIF: measurement of the angular distribution of 23Na + 40Ca elastic scattering

Wei Nan· Bing Guo· Cheng-Jian Lin,2· Lei Yang · Dong-Xi Wang·Yang-Ping Shen · Bing Tang · Bao-Qun Cui · Tao Ge · Yin-Long Lyu ·Hui-Ming Jia· Yun-Ju Li · Chen Chen· Li-Hua Chen · Qi-Wen Fan ·Xin-Yue Li· Gang Lian · Jian-Cheng Liu · Tian-Peng Luo · Nan-Ru Ma ·Rui-Gang Ma · Xie Ma · Ying-Jun Ma · Wei-Ke Nan · Dan-Yang Pang·You-Bao Wang · Pei-Wei Wen · Feng Yang · Yong-Jin Yao,4·Sheng Zeng · Hao Zhang· Fu-Peng Zhong,2 · Shan-Hao Zhong,2 ·Zhi-Hong Li · Tian-Jue Zhang · Wei-Ping Liu · BRIF Collaboration

Abstract The reaction dynamics of exotic nuclei near the drip line is one of the main research topics of current interest. Elastic scattering is a useful probe for investigating the size and surface diffuseness of exotic nuclei. The development of rare isotope accelerators offers opportunities for such studies.To date,many relevant measurements have been performed at accelerators using the projectile fragmentation technique, while the measurements at accelerators using isotope separator on-line(ISOL)systems are still quite scarce. In this work, we present the first proof-of-principle experiment with a post-accelerated ISOL beam at the Beijing Radioactive Ion Beam Facility(BRIF) by measuring the angular distribution of elastic scattering for the stable nucleus 23Na from the doubly magic nucleus 40Ca at energies above the Coulomb barrier.The angular distribution measured by a silicon strip detector array in a scattering chamber using the ISOL beam at BRIF is in good agreement with that measured by the high-precision Q3D magnetic spectrograph using the non-ISOL beam at nearly the same energy. This work provides useful background for making BRIF a powerful tool for the investigation of the reaction dynamics of exotic nuclei.

Keywords BRIF · Exotic nuclei · Elastic scattering ·Angular distribution

1 Introduction

Light loosely bound nuclei near the drip line are characterized by very low nucleon binding energies, typically one order of magnitude smaller than those for their stable counterparts located along the β-stability valley.These nuclei can exhibit exotic properties, such as a halo structure.The reaction dynamics of light exotic nuclei near the drip line is one of the main research topics of current interest and has attracted considerable interest in the lowenergy nuclear physics community[1–3].Elastic scattering is a useful probe for investigating the size and surface diffuseness of exotic nuclei by comparing the similarities and differences in the angular distributions of the reactions induced by loosely bound and tightly bound nuclei [4].

To date, several measurements have been made of the elastic-scattering angular distributions of neutron-rich nuclei, such as the 2n-halo nuclei6He [5] and11Li [6],neutron skin nucleus8He [7, 8],8Li [9], and the 1n-halo nucleus11Be[10–12].In recent years,the elastic scattering of proton-rich nuclei has also been investigated (e.g.,7Be,8B,9C+Pb[4,13,14],17F+12C and14N[15],17F+58Ni[16],17F +89Y [17], and17F +208Pb [18, 19]). These experiments have greatly deepened our understanding of the reaction dynamics and their interplay with the exotic structure of weakly bound nuclei. However, more investigations are needed.

The development of rare isotope accelerators offers opportunities to explore the structure of unstable exotic nuclei. There are two rare complementary isotope accelerators in China. One is the Radioactive Ion Beam Line in Lanzhou (RIBLL) [20] using the projectile fragmentation(PF) technique, which was established by the Institute of Modern Physics, Chinese Academy of Sciences. Since the delivery of the first beam in 1997, a series of experiments have been conducted for the study of, for example, the clustering structure in neutron-rich nuclei [21, 22], twoproton emission in proton-rich nuclei [23, 24], and revalidation of the isobaric multiplet mass equation [25]. In addition, the elastic-scattering angular distributions of a few proton-rich nuclei [4, 13, 17] and the 1n-halo nucleus11Be[12]have been measured using silicon detector arrays[26, 27] at RIBLL. The other accelerator is the Beijing Radioactive Ion Beam Facility (BRIF) [28, 29] using the isotope separator on-line (ISOL) technique, which was established by the China Institute of Atomic Energy.BRIF consists of a 100-MeV 200-μA compact proton cyclotron[30], an ISOL system with a mass resolution of 20,000[31], and a 13-MV tandem accelerator for post-acceleration. BRIF was commissioned in 2015 and successfully produced a few unstable ion beams such as20，21，22Na and37，38K.Recently,the exotic β–γ–α decay mode was directly observed for the first time with a pure20Na ISOL beam at BRIF [32].

BRIF is a potential high-precision facility for investigating the nuclear reaction dynamics of unstable nuclei,as it can deliver almost pure unstable ion beams.However,an experiment with a post-accelerated ISOL beam at BRIF has not been performed to date.Therefore,a proof-of-principle experiment with a post-accelerated stable23Na beam is highly desirable. For this purpose, the angular distribution of23Na +40Ca elastic scattering was measured using two techniques. One is based on a silicon detector array with a post-accelerated23Na beam using the ISOL technique at BRIF (ISOL beam); the other is based on a high-precision Q3D spectrograph with the23Na beam directly from the traditional negative-ion source and accelerated by the HI-13 tandem accelerator (non-ISOL beam). The excellent consistency of these two results demonstrates that BRIF can be a powerful tool for investigating the reaction dynamics of exotic nuclei.

2 Experimental setup and procedure

The experiment with the post-accelerated ISOL beam was performed at BRIF. First, a non-ISOL23Na beam directly from an ion source was accelerated by the HI-13 tandem accelerator as the pilot beam and transported to the R60 scattering target chamber to determine the beam optics. Second, the proton cyclotron served as the driving accelerator.The23Na beam was then produced with a 100-MeV 10-eμA proton beam from the cyclotron bombarding the MgO target. Reaction products diffusing out of the thick target were ionized by an ion source and separated by a two-stage ISOL system for subsequent post-acceleration.Finally, the ISOL23Na beam was accelerated by using the HI-13 tandem accelerator and transported to the R60 scattering target chamber for the angular distribution measurement with the same optical systems as used for the pilot beam. The energy and the current of the ISOL23Na beam were 83.25 MeV and 0.5 enA, respectively.

Fig. 1 (Color online) Experimental setup in the target chamber. The two MCPs and the QSD were used to identify the beam. A silicon detector array was used to detect emitted particles

The setup of the target chamber is illustrated in Fig. 1.Two micro-channel plates (MCPs), which can present a fast timing signal, were used to measure the time of flight(TOF)of the beam.A quadrant silicon detector(QSD)with a thickness of 1000 μm,which was placed at the end of the target chamber,was used to measure the total energy of the beam. The ISOL beam from BRIF can be confirmed by a combination of the TOF and energy.After the development of the23Na beam was confirmed, the upstream MCP and QSD were removed to avoid interference with the measurement of the angular distribution,while the downstream MCP was left to monitor the beam.The target was made by evaporation of natural CaF2with a thickness of 118 μg/cm2on a 200 μg/cm2thick Au foil. The silicon detector array was placed 10 cm downstream of the target. The detector array consists of four detector telescopes, as shown in Fig. 2. The first and second layers of each telescope are two single-sided silicon strip detectors (SSSDs)with thicknesses of 20 and 300 μm, respectively. Each SSSD has a typical energy resolution of 0.3% and has 16 strips with a width of 3 mm, spaced 0.1 mm apart. These two SSSDs were placed in the horizontal and vertical directions, respectively. The third layer is a QSD with a thickness of 1000 μm and an area of 50×50 mm2for potential light reaction products such as protons and α particles. Such a configuration can identify reaction products, including light and heavy ions. The angular coverage range of the present detector array in the laboratory system ranges from 10.2°to 39.6°, as shown in Fig. 3.

Fig.2 (Color online)Setup of the silicon detector array.The detector array consists of four detector telescopes. Each detector telescope contains three layers of silicon detectors with thicknesses of 20, 300,and 1000 μm, respectively. See the text for further details

Fig.3 (Color online)Angular coverage of the detector array.θ and φ are the angles used in the spherical coordinate system. The array covers the scattering angle θ, ranging from 10.2° to 39.6°

In this experiment, the energy of the23Na beam at the center of the target was 82.8 MeV.The scattered23Na ions were detected in the first two layers of the telescope. The 20-μm-thick SSSD was used for the measurement of energy loss ΔE, while a 300-μm-thick SSSD was used to measure the residual energy Er. The experimental spectra of the scattered23Na particles from40Ca and197Au are shown in Fig. 4. Both the two-dimensional spectrum of energy loss versus the total energy and the one-dimensional spectrum of the total energy are presented. The23Na particles from40Ca can be clearly distinguished from those from197Au.

To verify the ISOL-based technique at BRIF, the same angular distribution was also measured with a well-developed technique using a high-precision Q3D spectrograph with the non-ISOL23Na beam directly from the traditional negative-ion source and accelerated by the HI-13 tandem accelerator at the China Institute of Atomic Energy. The experimental setup and procedures were identical to those reported in our previous work [33, 34]. The experimental target was made by evaporation of natural CaF2with a thickness of 18 μg/cm2on a 30 μg/cm2thick Au foil. In this experiment,the energy of the23Na beam was 84 MeV,and its energy at the center of the target was 83.9 MeV(which was almost the same as the measurement at BRIF).

3 Data analysis and results

The differential cross section of a reaction can be expressed as

Fig.4 (Color online)Energy spectra of the scattered 23Na particles from 40Ca and 197Au.a Two-dimensional spectrum of energy loss ΔE versus total energy Etot. b One-dimensional spectrum of total energy

where N and I represent the numbers of emitted ions and incident ions,respectively,Nsdenotes the number of target atoms per unit area,and Ω represents the solid angle.In the present work, we used a relative measurement method to reduce the uncertainties from the solid angle and beam intensity. The cross section of23Na +197Au elastic scattering at the present energy is equal to the Rutherford cross section; therefore, the ratio of the measured23Na +40Ca elastic-scattering cross section to the corresponding Rutherford cross section can be calculated by using

In Fig. 5,we show the experimental angular distribution of23Na +40Ca elastic scattering with the ISOL-based technique at BRIF and a well-developed technique at a high-precision Q3D spectrograph,together with the optical model calculations with the single-folding potential [35].These two experimental results were in good agreement.This presents strong evidence that BRIF can be used for such measurements.

Fig. 5 (Color online) Angular distribution of 23Na + 40Ca elastic scattering. The red points are the results obtained using the ISOLbased technique at BRIF, while the blue points represent those obtained with the well-developed technique using a high-precision Q3D spectrograph. The solid and dashed curves stand for the optical model (OM) calculations at 82.8 and 83.9 MeV, respectively

4 Conclusion and perspective

In this work, we performed the first proof-of-principle experiment with a post-accelerated23Na beam using the ISOL technique at BRIF (ISOL beam) by measuring the angular distribution of23Na +40Ca elastic scattering. In addition,we measured the same angular distribution with a well-developed technique using a high-precision Q3D spectrograph with a23Na beam from the HI-13 tandem accelerator (non-ISOL beam). These two results are in excellent agreement, demonstrating that BRIF can be a powerful tool for future investigation of the reaction dynamics of exotic nuclei.

To the best of our knowledge, there are no elasticscattering data for unstable sodium isotopes20，21，22Na on the doubly magic nucleus40Ca. To explore the exotic properties of these unstable sodium isotopes, we plan to measure the angular distribution of21，22Na +40Ca elastic scattering at BRIF using the same technique described in this work in the near future.

Author ContributionsAll authors contributed to the study conception and design. Experiment was carried out by Wei Nan, Cheng-Jian Lin, Lei Yang, Dong-Xi Wang, Yang-Ping Shen, Hui-Ming Jia,Yun-Ju Li,and Xin-Yue Li.Targets were made by Qi-Wen Fan.Data analysis was performed by Wei Nan, Bing Guo, Cheng-Jian Lin,Yang-Ping Shen, Dan-Yang Pang, and Wei-Ping Liu. The ISOL beam was developed by Bing Tang, Bao-Qun Cui, Tao Ge, Yin-Long Lyu, Li-Hua Chen, Jian-Cheng Liu, Rui-Gang Ma, Xie Ma,Ying-Jun Ma, and Tian-Jue Zhang. The first draft of the manuscript was written by Wei Nan and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.